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Chapter 7 presents the attempted synthesis of a series of new co crystals, with components based on those of 4 methylpyridine pentachlorophenol; the successful products were found to possess medium length hydrogen bonds. Variable temperature diffraction studies for one of these products are discussed and show that it undergoes a phase transition on cooling resulting from slight rotations of its components. Chapter 8 gives the main conclusions of this thesis and outlines a number of opportunities for further work.

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